The group was founded in 2006 by Daan Blom (D44N) and Martijn Verlinden (Kipkillah), who were previously active in the music collective BAF Soundsystem. Charly & Gallus was the first dubstep group and liveset in the Netherlands. The band played at Lowlands in 2006 and at Noorderslag in 2007.  They won the Grand Prix of Zuid-Holland in 2008 and were selected for the semi-finals of the Grand Prix Netherlands in 2009. In May 2009 the group released the album Chemical Solutions. The record was called a little gem in a review of 3VOOR12. In 2010 Charly & Gallus played as well as 2562 in Vancouver (Canada) during the festival “CODE Live Night Life” of the Olympic Games.
On February 26, 2010 the compilation CD / DVD Antilounge 7 was presented, with the videoclip Nanomat. In August 2011 and 2012 Charly & Gallus were at the Sziget Festival in Hungary.